Solvent effects over optical properties of a two-level molecular system

J. L. Paz; M. Gorayeb; A. J. Hernandez

doi:10.1117/12.590726

21 October 2004 Solvent effects over optical properties of a two-level molecular system

J. L. Paz, M. Gorayeb, A. J. Hernandez

Proceedings Volume 5622, 5th Iberoamerican Meeting on Optics and 8th Latin American Meeting on Optics, Lasers, and Their Applications; (2004) https://doi.org/10.1117/12.590726
Event: 5th Iberoamerican Meeting on Optics and 8th Latin American Meeting on Optics, Lasers, and Their Applications, 2004, Porlamar, Venezuela

Abstract

The solvent effects over optical properties of a two level system in presence of an electromagnetic field was modeled in this work. The system-field interaction was considered by using the dipolar-electric approximation, assuming negligible the molecular permanent dipole moments. The solvent effects were included in the formalism in a stochastic form, through the induced shifts over the Bohr molecular frequency. The coherence was calculated from the optical stochastic Bloch equations (OSBE), and later, it was averaged over all realizations of the stochastic molecular variable. To do that, it was applied the convolution theorem, which was resolved using direct and inverse Fourier transforms.

Citation Download Citation

J. L. Paz, M. Gorayeb, and A. J. Hernandez "Solvent effects over optical properties of a two-level molecular system", Proc. SPIE 5622, 5th Iberoamerican Meeting on Optics and 8th Latin American Meeting on Optics, Lasers, and Their Applications, (21 October 2004); https://doi.org/10.1117/12.590726

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