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Interfacial electron transfer (IET) dynamics have been measured in a series of dye-sensitized metal oxides commonly using in water splitting dye-sensitized photoelectrochemical cells using optical-pump terahertz-probe spectroscopy. The IET dynamics were compared using a model that allows for the relative contributions of injection from the singlet and triplet excited states of the dye to be distinguished. In addition, we present a newly developed method for performing terahertz (THz) measurements under potentiostatic control (i.e., THz spectroelectrochemistry).
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Charles A. Schmuttenmaer, Jacob A. Spies, Coleen T. Nemes, John R. Swierk, "Interfacial electron transfer in dye-sensitized mixed metal oxides for water splitting," Proc. SPIE 10983, Next-Generation Spectroscopic Technologies XII, 109830R (13 May 2019); https://doi.org/10.1117/12.2522079