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Excitations in spatially indirect transitions feature such as excitons in type-II heterostructures or charge-transfer excitations in molecular crystals feature a permanent dipole moment which influences the transition dipole moments commonly probed by optical spectroscopy. Epitaxially grown III-V quantum heterostructures featuring suitable band alignments are ideal model systems to study the interplay between the two. Selected topics discussed include the AC Stark effect and signatures of spatially indirect coherent biexciton states as well as the potential for coherent optical current injection dynamics.
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Markus Stein, Felix Schäfer, Daniel Anders, Jan H. Littmnann, Michael Zengel, Kerstin Volz, Sangam Chatterjee, "Coherent optical nonlinearities in model type-II heterostructures," Proc. SPIE PC12884, Ultrafast Phenomena and Nanophotonics XXVIII, PC128840A (9 March 2024); https://doi.org/10.1117/12.3002331