The Orion facility is used mainly for studying high energy density physics. It has ten “long” pulse UV laser beams, two “short” pulse Petawatt beams and ancillary beams for probing of the experimental conditions. Occasionally experimental teams are requested to perform dedicated shots of a given configuration to obtain information on laser target fragments and their effects on surfaces within the target chamber. After these test shots witness plate surfaces were inspected by optical microscopy so that palliative measures could be taken or modifications to the experiment undertaken to minimize any deleterious effects on laser optics or diagnostic instrumentation.
Typically, plasma physics targets are of millimeter or sub millimeter dimensions and use an irradiance of ~1016 W/cm2 in nanosecond [“long”] pulses or ~1021 W/cm2 for “short” [~500fs] pulse lengths. These conditions lead to target and target mount materials being raised to temperatures that cause changes from the solid state into liquid, gaseous and plasma conditions. Matter from the altered states are then subsequently ejected from the originally solid target location and are distributed in space with a variety of masses and velocities and form layers or regions of contamination, some of which may be deposited on sensitive laser or X ray optical surfaces. If low energy densities are used then there is insufficient energy to change the state of the target and a plume of solid fragments is emitted by the target.
The use of solid targets irradiated in a vacuum target chamber by focussed high energy, high power laser beams to study the properties of matter at high densities, pressures and temperatures are well known. An undesirable side effect of these interactions is the generation of plumes of solid, liquid and gaseous matter which move away from the target and coat or physically damage surfaces within the target chamber. The largest aperture surfaces in these chambers are usually the large, high specification optical components used to produce the extreme conditions being studied [e.g. large aperture off axis parabolas, aspheric lenses, X ray optics and planar debris shields]. In order to study these plumes and the effects that they produce a set of dedicated experiments were performed to evaluate target by product coating distributions and particle velocities by a combined diagnostic instrument that utilised metal witness plates, polymer witness plates, fibre velocimetry and low density foam particle catchers.
When lasers are used to produce high temperature, high density plasmas from solid targets it is inevitable that the targets
are turned into a variety of products [gas, liquid, solid, sub-atomic particles and electromagnetic radiation] that are
distributed around the surfaces of the vacuum chamber used to field such experiments. These by products are produced
in plumes of debris and shrapnel that depend on the irradiation conditions, target materials and target geometry. We have
monitored the distribution of such plumes by witness plates and used microscopy, photography and spectrophotometry to
determine the physical state of material in the plumes and the spatial distribution from various target geometries. The
impact of this material on the operations of laser optics and plasma physics diagnostics is discussed.
Since the late 1990s staff at national laboratories have been studying the effects of high energy focussed laser beams
[>100J] on a variety of plasma physics targets to understand the disassembly of targets and their effects on target
chamber surfaces. Target geometries have included metal foils, polymer foils, metal cylinders or cones, gas bags, metal
wires and complex geometries of combinations of the above. The post shot target remnants have been studied by both
optical microscopy and scanning electron microscopy. The morphology of exposed targets indicated phase changes and
other physical phenomena [shock, spall, crater formation and material ejection]. Pre and post weighing of the targets has
been used to determine mass lost from the target. Initially most of the material distribution analysis was performed by
catching target by-products with glass or silica witness plates. Spatial and image analysis of micrographs has been used
to measure angular distributions of material and its form. Spectrophotometry of the exposed witness plates in the UVVis-
NIR region allowed transmission spectra to be determined and the reduction of transmittance at the laser
wavelengths of interest. It also allowed estimation of average debris thickness. Shrapnel size and velocity has been
studied by capturing fragments in silica aerogels. One unexpected aspect of studying the witness plates was the
identification of secondary emissions from solid surfaces close to the irradiated target, this showed that the near
environment of the target is also important in determining overall material distributions. We have been fortunate to find
interested collaborators at other UK, European and US laboratories that have brought considerable insight into target
disassembly processes and palliative measures.
All laser targets subjected to heating by focused energetic lasers for the study of high temperature plasmas produce
shrapnel, debris or radiation directly or indirectly that impact and coat the optics, instruments and surfaces used in the
vacuum chambers employed for such studies. We describe the spatial distributions of the target ejecta arising from
various configurations of thin walled metal cylinder targets and their mechanical mounting systems that have been
deployed on the Helen and ZBeamlet lasers. We also demonstrate how this data can be used to evaluate threats to optical
surfaces and ancillary instruments in high energy, high power laser systems. The methods used for characterizing and
quantifying material plumes will also be described.
In preparation for experiments on the ORION laser facility, a number of investigations have been performed to
characterise debris and shrapnel plumes arising from laser target interactions. These interactions may arise from the use
of long [ns] pulse or short [ps] pulse laser beams with mainly solid targets. Plume characteristics depend on the target
material and geometry. We describe interactions with metal or polymer targets and geometries including planar foils,
cylinders, wires, or complex combinations. Characterisation techniques were based mainly on glass witness plates or
aerogel catchers with subsequent analysis by optical or electron microscopy, spectro-photometry, and image analysis.
Chirped pulse amplification [CPA] has been implemented on laser facilities to produce high irradiance conditions in a
vacuum chamber for the study of novel plasma physics processes. When such focussed laser beams interact with solid
targets, the material is disrupted and leads to ejecta as solids, liquids, vapours and radiation. These target by-products can
degrade and damage optical or diagnostic surfaces in the interaction chamber. This paper describes the effects of such
emissions on surfaces by the use of metrology, microscopy, image processing, fragment capture in foams and autoradiography.
Target plume divergence is discussed so that precautions for future experiments can be evaluated.
The performance of plasma mirrors has been characterised on the HELEN laser infra-red, chirped pulse
amplification [CPA] beam line. This laser produced pulse energies up to 100J with pulse lengths of ~500fs. Plasma
mirrors are initially low reflectance surfaces that transmit low intensity light but produce a reflecting plasma surface
when exposed to high irradiance beams. Typically they are formed by transparent substrates at the laser wavelength
and have been used either uncoated or with anti-reflection coatings. The coatings evaluated in these experiments
were either multi-layer dielectrics or single layer sol-gel silica. Some of the fused silica substrates were coated on
both faces, others were coated on the incident face only and a small number were used uncoated. The reflectance of
the plasma mirrors was measured as a function of incident energy. A vacuum compatible pyro-electric sensor in
conjunction with either a diffuser or neutral density filter was used to measure incident and reflected laser energy.
Both the diffuser and filter could suffer laser damage at the highest incident energies available. The morphology of
the damage of the different components and coating combinations was studied as a function of incident beam
energy. The mirrors were being investigated to prevent pre-pulse effects in plasma physics experiments and increase
the intensity contrast ratio of the laser beam incident onto solid targets. Their proximity to the laser target also
allowed them to block debris and shrapnel arising from the laser matter interaction in some directions. These
material emissions spread uncontrollably in the evacuated target chamber and may cause contamination of laser
optics and filters or radiation diagnostic instrumentation. The plasma mirror components were operated at 45
degrees angle of incidence and an average input beam diameter of 5.5 millimetres at the mirrors with incident beam
irradiances in the range 50 TW/cm2 to 540 TW/cm2. The reflected beams were focussed on to 10 micron thick,
10mm diameter metal foils and 3mm diameter polymer/metal targets with a thickness of 2 to 18 microns. The
subsequent debris and shrapnel effects were studied using post shot microscopy and photography.
In this paper we review contamination and damage that has occurred since the HELEN laser was converted for use
as a chirped pulse amplification (CPA) system. We concentrate on the largest components in the facility that
operated in a vacuum environment in the short pulse (500fs) parts of the system. This experience will be valuable for
planning commissioning and operations on the successor facility, ORION that is currently being constructed.
The optical components located in the vacuum sections will be described. We have an interest in laser-induced
damage and contamination from the long pulse only (~1ns), short pulse only (500fs) and combined regimes. For
most of the operations the CPA system has operated at a wavelength of 1053nm (1ω). Some experiments have also
been conducted with 527nm (2ω) CPA light derived by the use of a KDP doubling crystal. Damage to the infra red
pulse compression gratings has occurred infrequently with a minority of high-energy shots. Contamination of
multilayer dielectric plane turning mirrors has arisen from target disassembly. Focussing systems using off axis
parabolic mirrors have sustained contamination from debris and a dielectric protected silver reflector used for green
light suffered laser induced damage. Debris shields placed between the target and the parabolas have been used on
selected experiments. The shields were anti-reflection coated with single layer, sol gel silica. These shields became
contaminated on the target facing sides and in the case of 2ω operation also from blow off of the damaged mirror
coating that caused a two-pass transmission loss in the system.
A number of characterisation methods were used to evaluate and quantify the damage and contamination. These
include macroscopic photography, microscopy, reflectometry and transmission spectroscopy.
The performance of sacrificial and plasma mirrors has been investigated on the HELEN laser chirped pulse
amplification [CPA] beam line. Sacrificial mirrors are initially highly reflective surfaces that degrade during the
course of a pulsed laser experiment. They are being considered for protecting the off axis parabolic surfaces used to
focus CPA lasers from plasma physics target generated debris and shrapnel. Plasma mirrors are initially low
reflectivity surfaces that transmit low intensity beams but produce a reflecting plasma surface during the course of
the laser pulse. They are being investigated to prevent prepulse effects in plasma physics experiments and increase
the contrast ratio of the incident laser beam.The sacrificial mirrors were operated at 45 degrees angle of incidence
and an average input beam diameter of ~14 mm with intensities in the range 8 TW/cm2 to 44 TW/cm2. Dielectric
protected silver and gold coatings as well as dielectric multi layers were studied as the mirror surfaces for directing
all of the short pulse [500fs] laser beams onto tantalum foil targets of 10 microns thickness. Proton emissions from
the foils monitored by radiochromic film were used to evaluate the beam irradiance achieved from the mirror
surfaces. Glass witness plates were used to evaluate debris and shrapnel emissions from the mirror surfaces, the
diagnostics and the target foils. The plasma mirrors were operated in a similar configuration but with beam
diameters of ~8mm and irradiances of 57 TW/cm2 to 235 TW/cm2. Uncoated and sol gel anti-reflection coated
fused silica were used as the high intensity mirror surfaces. The influence of surface coating on laser damage
morphology will be described as well as post shot inspection of debris distributions.
The implementation of CPA on one of the HELEN laser beams has prompted the need for investigations into the survivability of reflective and refractive focussing optics during laser-target interaction experiments. These experiments generate debris that has the potential to contaminate the optics cumulatively over time, and in some cases produce high-energy shrapnel, which may damage the focussing optics on an individual shot. Inserting a thin (2mm) coated glass substrate into the beam path allows for its use as a mitigation shield by obstructing the line of sight for debris and shrapnel to travel directly from the target to the focussing optic. A series of experiments have been conducted using such debris shields on the CPA beam line at the HELEN laser facility AWE, Aldermaston. The influence of the debris shield on focal spot behaviour will be described. Directionality and contamination density of target debris has been characterised by the use of thin glass witness plates and post-shot inspection by optical microscopy.
AWE has operated lasers for studying the properties of materials at high temperatures and pressures since the early 1970s [1]. A brief review of those facilities will be given along with a description of the changes to HELEN in the period 2003 - 2005 to enable it to provide both chirped pulse amplification [CPA] pulses and nanosecond pulses to laser targets simultaneously. The CPA beam is now giving laser pulses of typically 70 Joules in 500 femtoseconds. As a necessary part of operating such a system it has been necessary to study how laser-target debris is distributed from both long and short pulse interactions so that the contamination or degradation of focussing optics during operational activities is minimised. The short pulse experiments and the characteristics of debris fields emanating from laser targets will be described. Damage thresholds were established for coated and uncoated debris shields with millimetre to centimetre size beams. Future developments of the laser facilities at AWE in this decade will also be described as well as possible debris mitigation options that may be employed.
Progress in building high-energy, short pulse laser systems with peak powers in the 100 to 1000 TW regime and applying them to plasma physics experiments has highlighted the need for debris mitigation solutions compatible with high intensity pulses [1]. Mitigation schemes ideally need to protect focusing optics for a number of laser pulses at reasonable cost without degrading beam quality. In this paper we describe preliminary experiments performed at the VULCAN laser facility to address some of these issues. The short pulse beam was passed through a thin optical shield at intensities up to 4 x 1012 W/cm2. The transmission of the shield was measured as a function of intensity along with the near and far field beam quality. Transmission losses occurred at the highest intensities used and these were related to the start of laser damage of the shield. The morphology of the damage features on the surface and in the bulk material was studied by a combination of white light interferometry as well as optical and scanning electron microscopy.
The use of large aperture high power lasers to study plasmas formed from solid targets is well known. In this paper we consider the effects of second harmonic Neodymium laser radiation [527 nm] on optical surfaces that have been contaminated by solid shrapnel and liquid or gaseous debris arising from the use of laser irradiated solid targets. In typical operations large lasers use debris shields to protect expensive aspheric lenses from optical and mechanical damage. These debris shields have a finite lifetime before they need to be replaced. Criteria for replacement have often been derived empirically from operational experience of evacuated target chambers and may be based on transmission, reflectivity, scatter or obscuration measurements. Here we describe and characterize the debris produced from targets based on gas bags, spall packages and gold halfraums captured on fused silica borosilicate plates. The influence of contamination levels and the physical form of debris on laser beams of various fluences was measured. Laser cleaning, damage thresholds and growth rates were investigated and the techniques are described.
This paper discusses laser beam, debris and shrapnel induced damage on optical components of a pulsed high power Neodymium laser system. Quantitative and qualitative investigations of the nature of laser damage on optical components and coatings that form the laser system are presented as well as investigations of debris and shrapnel induced damage on sol gel anti reflective coated optical components that surround the taget. In addition laser target debris and shrapnel induced damaged on sol gel thin film coatings have been studied where optical transmission was measured using an Ultra Violet Visible spectrophotometer before and after coated optics were used in the system and experienced damage. The problem with understanding causes of each type of damage is difficult because many processes occur simultaneously in an operational target chamber. Also investigated was the effect of low irradiance laser light at removing debris, and the rate of laser damage growth on contaminated HELEN optics, with number of laser shots.
This paper discusses the development of sol-gel thin films at AWE with respect to the formation of high reflectivity optical coatings. The use of such mirrors allows the separation of 1053 nm [1ω], 527 nm [2ω] and 351 nm [3ω] light from high power Neodymium laser systems before entering a target chamber and focusing onto a plasma physics target. The coating technique to achieve successful mirrors is discussed along with the analysis of the multilayers. Issues of scaling up from 50-mm diameter components to the coating of 150-mm square optics are reported along with the simultaneous achievement of high reflectivity, uniformity, wavefront preservation and high laser induced damage thresholds (LIDT).
The formation of thin film single layers and multilayers from sol-gel materials at room temperature inherently yields a coating with residual organic impurities and trapped solvent. Both of these features have the potential to act as initiators or secondary activators of laser damage. The laser induced damage threshold (LIDT) of single layer anti- reflective silica and single layer high index zirconia coatings have been assessed as a function of curing temperature. A coating of 200-nm thickness deposited by dip coating was exposed to elevated temperatures in an air atmosphere from 20 degree(s)C to 350 degree(s)C and cooled to room temperature and pressure (RTP) before testing. The effect of this rise in temperature on the LIDT is discussed. Ultra Violet-Visible transmission spectra of the thin films are also presented. A clear densification process was found to occur leading to both a change in thickness and refractive index as a function of temperature. The absence of this trend in the low index silica layer is believed to be a direct consequence of the different chemistry during formation as a similar solvent is used in both the high and low index layers. The implications of this with respect to the effect on multilayers are also discussed.
Anti-reflective thin films used on optics within the target chambers of high power lasers used for plasma physics experiments degrade significantly in use. The cause of this may not be attributed to any single influence. Coating from target debris, absorption of vacuum chamber vapors, and the exposure to vacuum conditions and X rays will all contribute. To simulate some of these conditions, sol-gel derived optical film ageing studies have been performed on a range of anti-reflective coatings over a 4-month period. Similarly the use of sol-gel High Reflectivity coatings for mirrors need to be durable and stable with time in their likely working environments. The coatings have been assessed with regard to their laser induced damage threshold (LIDT), transmission properties, refractive index and thickness at three wavelengths (355 nm, 532 nm and 1064 nm). Although exact replication of the conditions is impossible some of the parameters have been controlled including pressure and humidity as a function of time. We report on the changes experienced by these coatings under these conditions and discuss possible reasons for the observed trends and the effect this could have on coating selection.
Previous studies of for sol-gel coated multilayer UV mirrors have shown a significant decrease in laser induced damage threshold (LIDT) between the single component layer coatings and ten pair multilayer coatings. Further investigation has shown that the LIDT decreased rapidly after the first two pairs however no further decrease was seen with the subsequent deposition of more layers. In this paper, the effect on the LIDT of starting and finishing with high index material was assessed as a function of the number of layers. The effects on LIDT and environmental stability, i.e. the reaction to changes in temperature and pressure, of using a silica or Teflon half wave overcoat were also investigated. Different coating treatments, e.g. baking each layer applied to the substrate, were also investigated with the aim of improving both the LIDT and the number of layers which could be deposited, and hence the reflectivity of the mirrors, without the occurrence of crazing. Investigations into the damage morphologies were made and differences between the samples compared.
Teflon AF 1600 and 2400 have been used to make thin film coatings with excellent anti-reflective (AR) properties. Spin, dip, and meniscus coating techniques have all successfully formed single layer AT coatings. Multi-spin and dipping of the Teflon AF polymer revealed a close linear relationship between the number of layers and total thickness of the Teflon film. HFE7100 and Hexafluorobenzene were used as co-solvents to allow good control of the coating thickness by dilution allowing the dipping or spinning rate to remain at their optimum values. Significant differences were seen between these solvents with respect to coating quality. LIDT results are reported for the single layers AT coatings along wit surface properties and attempts to stack other materials onto the Teflon films.
Depth profiling using Dynamic Secondary Ion Mass Spectroscopy through multilayer coatings on fused silica substrates has revealed the effect of increasing the number of layers in the stack. Results are presented for both spin and dip coated multilayers and a significant difference in the interfacial boundary is seen between the two processes. Individual layer thicknesses were estimated using this technique and compared to values gained from UV-Visible spectroscopy. Depth profiling using SNMS of a thick 2-layer system also revealed the thickness of the layers and an indication of the intermixing between them. These measurements agreed well with UV-Vis data. A comparison between these depth-profiling techniques and previous work using AES/XPS depth profiling is discussed.
Previous results1 have shown that single layers of nitric or acetic acid stabilised zirconia and silica sol-gels have very high laser induced damage thresholds (LIDT). A significant decrease in the LIDT has been found when the materials are combined in layer pairs to form ultra violet mirrors. Investigations of possible causes of the lower LIDT will be reported. The effect of the coherent intensity enhancement at interfaces was tested by measuring the LIDT at 3 55nm on mirrors of different wavelength tuning. Three nine pair mirrors were used. These components are for use at 355nm and the first high reflector was specified at this wavelength. The other two components were made with high reflectivity at 300nm and 400nm and lower reflectivity at 355nm to check how the intensity ofthe internally reflected light would affect the LIDT.
Laser induced damage thresholds, measured using N-on-1 and R-on-1 testing, of single layer high index zirconia and hafnia coatings, derived from nitric or acetic acid stabilized sol-gel processing, are reported. Single layer acetic acid, nitric acid and base catalyzed silica sol-gel coatings have also been tested. The sol-gels were dip coated onto fused silica substrates at a rate of 3mm/s. The refractive index of the materials were measured using transmission spectra of multiple pairs of high and low refractive index materials. Absorption in the UV region was similarly measured with multiple layers of the same material and fitting to a Beer's law behavior. The high index materials used were zirconia or hafnia, the low index material was silica. The compatibility of the various combinations of high and low index materials for physical stacking without cracking, achieving high reflectivity and high damage thresholds are discussed and compared.
At the first ICF conference some of the present authors described advances towards low-index silica AR coatings and high-index zirconia HR coatings on fused silica for use at 1.06 micrometers , where silica and zirconia coatings showed good laser-induced damage thresholds. Here progress towards full 3(omega) mirrors at 351 nm using well defined sol-gels to produce the necessary SiO2-ZrO2 stacks is described in detail. Results suggest that these SiO2-ZrO2 stacks have higher laser damage resistance than previous ones and that MgF2 and Sc2O3 alternatives may improve the mirrors still further. The nature of damage caused to these coatings by Nd-YAG laser at 355 nm operating with pulses of 11 ns duration and a beam 1 mm in diameter is also reported.
Zirconia and silica sol gels have been spin and dip coated on 50mm diameter fused silica substrates to produce 351nm HR multilayer stacks and very high laser damage thresholds. Multilayer coating design software has been used to estimate the refractive indices of individual layers. A spectrophotometer has been used to evaluate the absorption coefficient of the zirconia layers in the UV region. The coatings were typically found to craze after about 6 to 9 layer pairs had ben deposited. Laser damage thresholds up to 8J/cm2 have been measured using a frequency tripled Nd:YAG laser at 351nm and 0.7ns pulse duration using constant and ramped fluence sequences. The coatings and laser damage morphologies have been evaluated using optical, interferometric and electron microscope techniques.
Preliminary investigations of a potential broad band oscillator for the HELEN laser facility and its proposed upgrade are described. The reasons for the need of broad bandwidth and the choice of commercial technology to achieve it are discussed. The characterization of the device and the diagnostics used for the investigations are described. Small signal amplification of the bandwidth by a glass amplifier was also performed along with investigations of the effect of various bandwidths on the far field beam quality when using random phase plates.
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