We have studied dispersion of surface plasmon polaritons (SPPs) in the Kretcshmann’s geometry (prism/Ag/dye-doped polymer) in weak, intermediate, and ultra-strong exciton-plasmon coupling regimes. The dispersion curves obtained in the reflection experiment, were in a good agreement with the simple model predictions at small concentrations of dye (Rh590 and Rh610) in the polymer (PMMA). At the same time, a highly unusual multi-segment ladder-like dispersion curves were observed at extra-large dye concentrations. The dispersion curves observed in polymers co-doped with two dyes (Rh590 and Rh610) suggest strong coupling of excitons in the Kretchmann’s geometry. Acknowledgments: NSF 1856515, DOE/NNSA DE-NA0004007.
We have studied dispersion of surface plasmon polaritons (SPPs) in the Kretcshmann’s geometry (prism/Ag/dye-doped polymer) in weak and strong exciton-plasmon coupling regimes. In reflection, the dispersion curves were in a good agreement with simple model predictions at small concentrations of the dye (R6G) in the polymer (PMMA). At the same time, highly unusual multi-segment ladder-like dispersion curves were observed at large dye concentrations. To describe this behavior, we upgraded the theoretical model taking into account strong exciton-plasmon coupling. The dispersion curves obtained in emission experiments were strongly different from those in reflection and did not seem to be affected by the strong coupling.
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