We demonstrate the laser induced forward transfer of fluorescent dye solution thin films with different viscosity by employing a single 532-nm nanosecond optical vortex pulse. Upon irradiating the laser pulse, a single microdroplet is ejected from the donor film, and it is deposited onto a receiver substrate. Well-aligned microdots with the same diameter were printed on the substrate with optical vortex, whereas the production of microdots in uniform size was prevented with a conventional Gaussian beam. In addition, we demonstrate the microprinting of a number of droplets by optical vortex.
We demonstrate the creation of a microdroplet with a plasmonic Au nanoparticle core by employing the optical vortex
laser-induced forward transfer technology. The single plasmonic nanoparticle in the microdroplet is printed as a plasmonic
nanocore on a receiver substrate with a spatial resolution beyond the diffraction limit. This phenomenon manifests that the
optical vortex traps three-dimensionally only a suspended single Au nanoparticle in its dark core by its repulsive force
owing to plasmonic resonance, and it has the potential to realize a myriad of plasmonic structured materials.
Plasmonic nanostructures enable us to enhance light fields at nanoscale beyond diffraction limit, thereby offering us metamaterials and plasmonic crystals to realize exotic light-matter interactions, including negative refractive index, invisible cloaking, and perfect absorption.
We here demonstrate, for the first time to be the best of our knowledge, the creation of a single water microdroplet with a single plasmonic Au nanoparticle (~150 nm) core (plasmonic nanocore) by employing the optical vortex induced forward transfer. The microdroplet can be easily trapped to form a single plasmonic nanocore on a receiver substrate with a spatial resolution beyond the diffraction limit. Going beyond conventional fabrication processes for plasmonic structures, such as lithography technologies based on electron and ion beams, such plasmonic nanocore formation in a water microdroplet should offer us new fabrication technology for plasmonic structures.
We demonstrate successfully the creation of a microscale lead halide perovskite crystal by employing optical vortex laser induced forward transfer (OV-LIFT) technology. The created microscale crystals exhibit efficient visible (cyan~green~red) fluorescence with a lifetime of ~7 ns.
We discover an entirely novel phenomenon, so-called the formation of curved “spin-jet”, in which an irradiated fractional optical vortex provides a donor film non-axisymmetric torque to form a “spin-jet” with a curved trajectory. This phenomenon allows the development of a novel pattering technology to scan the ejected donor dots without any mechanical systems.
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