Josephson-junction-based low temperature rapid single flux quantum (RSFQ) superconducting electronics is already a mature technology, which is expected to perform at speeds exceeding 100 GHz [1]. However, the RSFQ technology still lacks a fast enough output interface between its operating circuit temperature T = 4.2 K and the room temperature electronic environment. RSFQ circuits work at liquid helium temperatures and the direct interconnection of these circuits and room temperature circuits using, e.g., copper transmission lines would consume too much of the cooling power [2]. To solve this problem a magneto-optical (MO) output interface has been proposed [3], in which the output current pulse from the RSFQ circuit is converted into an optical pulse and delivered to room temperature readout circuitry via an optical fiber.
The temporal output of a Ti:Sapphire laser system has been optimized using an acousto-optic programmable dispersive filter and a genetic algorithm. In-situ recording the evolution of spectral phase, amplitude and temporal pulse profile for each iteration of the algorithm using SPIDER shows that we are able to lock the spectral phase of the laser pulse within a narrow margin. By using the second harmonic of the CPA laser as feedback for the genetic algorithm, it has been demonstrated that severe mismatch between the compressor and stretcher can be compensated for in a short period of time.
A novel subpicosecond pulse radiolysis experimental system has been developed in Terawatt Ultrafast High Field
Facility (TUHFF) at Argonne National Laboratory. TUHFF houses a 20 TW Ti:sapphire laser system that generates 2.5
nC sub-picosecond pulses of 4-25 MeV electrons at 10 Hz using laser wakefield acceleration. The system has been
optimized for chemical studies. The subpicosecond electron pulses were used to generate hydrated electrons in pulse
radiolysis of liquid water. Preliminary transient absorption spectroscopy data with picosecond resolution is presented.
A terawatt tabletop laser wakefield acceleration source of relativistic electrons has been developed in our Terawatt Ultrafast High Field Facility (TUHFF). The preliminary results for ultrafast radiolysis of liquid water using this femtosecond electron source are presented. A TUHFF based femtosecond x-ray source is proposed. Thomson scattering of the accelerated electrons off a counterpropagating terawatt laser beam will be used to generate keV x-ray photons. The expected parameters of this x-ray source have been estimated. The short pulse duration, high flux, and good collimation of the resulting x-ray beam would be conducive for ultrafast time-resolved x-ray absorption studies of short-lived transient species in gases, liquids, and solids. It is argued that the solvation dynamics of Br atoms generated in photoinduced electron detachment from aqueous bromide would make a convenient choice for the first pump-probe experiment using this x-ray source.
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