We present an algorithm for the rapid retrieval of the carbon dioxide total column amounts (XCO2) using short wave infrared (SWIR) spectra of the reflected sunlight measured from space. The algorithm takes advantage of the combined processing of observational data from two different satellite missions. For the algorithm implementation we adopted the previously developed EOF (Empirical Orthogonal Functions)-based approach that exploits regression relations of the principal components of the measured spectra with target XCO2 values. In the original algorithm version the regression coefficients were derived by using training sets of collocated satellite and ground-based observations (ground-based observations were treated as “true values”). In this paper we implemented similar approach in which training set for one satellite mission is created using collocated observations of the another “reference” space mission simultaneously on-orbit (in this case XCO2 retrievals of the “reference” mission were treated as “true values”). This approach enables rapid data processing of the new satellite missions omitting expensive and time consuming stage of retrieval algorithm development. The feasibility of the approach was tested by joint processing of GOSAT and OCO-2 observation data. For the analysis of the algorithm precision/accuracy characteristics we used the collocated observations from the Total Carbon Column Observing Network (TCCON).
It is reported that the sensitivities of the short wavelength infrared bands of Thermal And Near-infrared Sensor for carbon Observation (TANSO) - Fourier Transform Spectrometer (FTS) on Greenhouse gases Observing SATellite (GOSAT) have been degraded with the wavenumber dependencies1. These degradations affect to the XCO2 and XCH4 retrievals, so they have to be correctly considered in the retrieval algorithm. In this work, we developed a new algorithm to evaluate these degradations from on-orbit solar calibration spectra using principal component analysis. The effectiveness of this algorithm is to be able to distinguish the time-dependent components of the spectral variability from the independent ones. This possibly enables us to evaluate the temporal change of sensitivity more precisely. The degradation models were constructed by decomposing spectra, fitting principal components scores using the appropriate functions, and reconstructing those functions. The first components of the decomposed eigenvectors have less spectral dependencies for each band, because they are due to the angular dependency of reflectance of the diffuser plate. On the other hand, the other components have significant spectral dependencies and their temporal variabilities do not correspond to that of the first component. This fact indicates that the components have to be separately considered to construct the degradation models of TANSO-FTS.
We present further development of the empirical orthogonal functions (EOF)-based retrieval algorithm. The algorithm output is a regression formula that relates principal components of the reflected sunlight spectra with CO2 total column amount. The algorithm was implemented and tested for the observations from the Japanese satellite Greenhouse gases Observing Satellite (GOSAT). Training of the EOF-based algorithm with the collocated ground-based and space-borne data (e.g., Total Carbon Column Observing Network and GOSAT observations, respectively) was shown to impose some errors that were interpreted as a result of implicit averaging over the collocation area. Alternative training with the small subset (∼5 % to 10%) of the full-physics algorithm is free of such errors; however, this option requires additional filtering of the space-borne observations that are strongly affected by atmospheric light scattering. This filtering was implemented by the comparison of the EOF-regression estimates of surface pressure with corresponding meteorological data.
We present satellite-based data of the column-averaged dry air mole fraction of atmospheric carbon dioxide (XCO2) and methane (XCH4), which were derived from the radiance spectra measured by Greenhouse gases Observing SATellite (GOSAT). We have applied new version of the Photon path-length Probability Density Function (PPDF)-based
algorithm to estimate XCO2 and PPDF parameters. These parameters serve to allow for optical path modification due to
atmospheric light scattering and they are retrieved simultaneously with CO2 concentration using radiance spectra from
all available GOSAT short wave infrared (SWIR) bands (oxygen A-band, 1.6-μm, and 2.0-μm CO2 absorption bands). For the methane abundance, retrieved from 1.67-μm absorption band, we applied optical path correction based on PPDF parameters from 1.6-μm CO2 absorption band. Similarly to widely used CO2-proxy technique, this correction assumes identical light path modifications in 1.67-μm and 1.6-μm bands. This approach is believed to offer some advantages over the proxy technique since it does not use any prior assumptions on carbon dioxide concentrations. Both carbon dioxide and methane GOSAT retrievals were validated using ground-based Fourier Transform Spectrometer (FTS)
measurements provided by the Total Carbon Column Observing Network (TCCON). For XCO2 retrievals we found subppm station-to-station bias (GOSAT versus TCCON); single-scan precision of mostly below 2 ppm (0.5%); and
correlation coefficient for the Northern Hemisphere TCCON stations above 0.8. For XCH4 retrievals over TCCON sites
we found single-scan precision below 1 % and correlation coefficient above 0.8.
Inverse estimation of surface C02 fluxes is performed with atmospheric transport model using ground-based and GOSAT observations. The NIES-retrieved C02 column mixing (Xc02) and column averaging kernel are provided by GOSAT Level 2 product v. 2.0 and PPDF-DOAS method. Monthly mean C02 fluxes for 64 regions are estimated together with a global mean offset between GOSAT data and ground-based data. We used the fixed-lag Kalman filter to infer monthly fluxes for 42 sub-continental terrestrial regions and 22 oceanic basins. We estimate fluxes and compare results obtained by two inverse modeling approaches. In basic approach adopted in GOSAT Level4 product v. 2.01, we use aggregation of the GOSAT observations into monthly mean over 5x5 degree grids, fluxes are estimated independently for each region, and NIES atmospheric transport model is used for forward simulation. In the alternative method, the model-observation misfit is estimated for each observation separately and fluxes are spatially correlated using EOF analysis of the simulated flux variability similar to geostatistical approach, while transport simulation is enhanced by coupling with a Lagrangian transport model Flexpart. Both methods use using the same set of prior fluxes and region maps. Daily net ecosystem exchange (NEE) is predicted by the Vegetation Integrative Simulator for Trace gases (VISIT) optimized to match seasonal cycle of the atmospheric C02 . Monthly ocean-atmosphere C02 fluxes are produced with an ocean pC02 data assimilation system. Biomass burning fluxes were provided by the Global Fire Emissions Database (GFED); and monthly fossil fuel C02 emissions are estimated with ODIAC inventory. The results of analyzing one year of the GOSAT data suggest that when both GOSAT and ground-based data are used together, fluxes in tropical and other remote regions with lower associated uncertainties are obtained than in the analysis using only ground-based data. With version 2.0 of L2 Xc02 the fluxes appear reasonable for many regions and seasons, however there is a need for improving the L2 bias correction, data filtering and the inverse modeling method to reduce estimated flux anomalies visible in some areas. We also observe that application of spatial flux correlations with EOF based approach reduces flux anomalies.
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